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And Secrest, D. (1981). J. Chem. Phys. 75, 3967. Engelking, P. C, and Smith, A. L. (1975). Chem. Phys. Lett. 36, 21. Evenson, K. , Wells, J. , and Radford, H. E. (1970). Phys. Rev. Lett. 25, 199. Fehsenfeld, F. C. (1975a). Int. J. Mass Spectrom. Ion Phys. 16, 151. Fehsenfeld, F. C. (1975b). In "Interactions Between Ions and Molecules" (P. ), p. 387. Plenum Press, New York. Ferguson, E. , Fehsenfeld, F. C , and Schmeltekopf, A. L. (1969). Adv. At. Mol. Phys. 5, 1. Gauyacq, J. P. (1982). J. Phys.

3, and these spectra are inverted as described earlier to obtain vibrational populations. In this calculation, a room temperature Boltzmann distribution is assumed, and the positions, line strengths, and spectral resolution are specified. The average results of the relative vibrational populations 22 BIERBAUM, ELLISON, AND LEONE after correction for radiative cascading are displayed in Table III (Weisshaar et al, 1981). The relative populations can be used to generate the complete product distribution if the v = 0 population is known.

FLOWING AFTERGLOW STUDIES OF ION REACTION DYNAMICS 21 As indicated in Table III, the exothermicities of the ion reactions are comparable to their neutral analogs but the rate constants are roughly two or three orders of magnitude larger. The fast rates of ion-molecule reactions are generally attributed to the presence of the large attractive well. In general, both the ion and neutral reactions have a tendency to dispose of a large fraction of the exothermicity into product vibration. , 1981): er + ΗΒΓ, H I -► HCI(Ü) + B r , r (2) and F" + HCl, HBr, HI -> HF(u) + CT, Br", I".

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